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lt in Production and Decay of an Isotope, 278 113, of the 113 th Kosuke Morita Superheavy Element Laboratory RIKEN Nishina Center for Accelerator-Based Science, RIKEN 1 2013/1/15 RIBF SEMINAR

New Result in Production and Decay of an Isotope, 278 113, of the 113 th Element Kosuke Morita

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New Result in Production and Decay of an Isotope, 278 113, of the 113 th Element Kosuke Morita Superheavy Element Laboratory RIKEN Nishina Center for Accelerator-Based Science, RIKEN. The Periodic Table has been evolving!. Region of interest. 120?. 114?. new nuclides: ~ 40/year . - PowerPoint PPT Presentation

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Page 1: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

New Result in Production and Decay of an Isotope, 278113, of the 113th Element

Kosuke Morita

Superheavy Element LaboratoryRIKEN Nishina Center for Accelerator-Based Science, RIKEN

12013/1/15 RIBF SEMINAR

Page 2: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 2RIBF SEMINAR

Page 3: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

The Periodic Table has been evolving!

32013/1/15 RIBF SEMINAR

Page 4: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

N

Z

Region of interest

114?

184

120?

new nuclides: ~ 40/year

new element: ~ 0.3/year

42013/1/15 RIBF SEMINAR

Page 5: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

a b c d e f

a bc

de

f

V= Z1Z2e2

R

Pote

ntial

ene

rgy

Bf: fission barrier

Deformation or distance between two centers of fragments R

: saddle: scission

52013/1/15 RIBF SEMINAR

Page 6: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 6

deformation

Pote

ntial

ene

rgy

RIBF SEMINAR

Page 7: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Z=116

72013/1/15 RIBF SEMINAR

Page 8: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 8

spherical deformed (axially symmetric)

factorscalePRRn

nn :])(cos1[)(2

0

surfaceenergy

Coulombenergy

3/2

20

0 4

Aa

RE

S

S

)75

521(

),,(

23

22

0

32

S

S

E

E

3/1

2

0

220

53

AZa

ReZE

C

C

)4910

511(

),,(

23

22

0

32

C

C

E

E

0R )(R

)()(),( 3/123/2 AAZaAZNaAaAaZAB CiSV Weizsächer-Bethe

)2

1(52)()0( 0

002

223S

CSCS E

EEEEE b2 deformation only

)804.17,710.0(501

22)(

22

0

0

MeVaMeVaAZ

AZ

aa

EEfissilityx

SC

S

C

S

C

Page 9: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

deformation

Ener

gy

saddle

scission

9

Physics of heavy and superheavy nuclei

large scale nuclear transmutation quantum mechanical shell effect

2013/1/15 RIBF SEMINAR

Page 10: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Superheavy Element

10

age of the universe ~  4.3x1017 s

2013/1/15 RIBF SEMINAR

Page 11: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

11

120

119

118

117

116

115

114

113

112

Rg

Ds

Mt

Hs

Bh

Sg

Db

Rf

162 184

262

266

265264

262

261

261

260259

258

257 258 260259

260 261 262

263

262261

SHE

A

A

A

-decay

Spontaneous fission

b+ or EC decay

one end of nuclear chart ’84 -’ 94

2013/1/15 RIBF SEMINAR

Page 12: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

12

120

119

118

117

116

115

114

113

112

Rg

Ds

Mt

Hs

Bh

Sg

Db

Rf

162 184

262

266

265264

262

261

261

260259

258

257 258 260259

260 261 262

263

262261 263

265 266

267266

259

264

269 270 271

267266

262

272

268

269 270 271

277

278

273

274

261

270

265

263

264

267

267 268

268

271 272

271

275 276

275

279 280

279

278

281

284 285 286

282

282

283 284

283

287 288 289 290286

287 288

290 291 292 293

294

SHE

A

A

A

-decay

Spontaneous fission

b+ or EC decay

one end of nuclear chart 2009

263

278

274

270

294293

290289

286285

282281

one end of nuclear chart 2010

2013/1/15 RIBF SEMINAR

Page 13: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Main Limitations of Various Approaches to SHE

Reaction Mode Proj. (Aproj)

Limitation Heaviest Nuclide

comment

(Z) (N)

multiplen-capture

n SF* of Fm isotopes 100 157 maybe possible in nature (r-process)

hot fusion(HI,xn);x=3-6Ucn≥40 MeV

≤34&48

small survival prob.(Gn/Gf very small)

118 176 N-rich beam often improves.(cf. 48Ca;warm fusion)

cold fusion(HI,xn);x=1,2Ucn ≤20 MeV

50-70 small fusion prob.(dynamical hindrance of fusion?)

113 165

transferreaction

≤22 lack of target heavier than 254Es**

103 159

*SF: spontaneous fission. cf. T1/2 of 258Fm158 ≈ 400 ms.**254Es(Z=99): T1/2 ≈ 276 day

132013/1/15 RIBF SEMINAR

Page 14: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Ring Cyclotron pamphlet 1986 First Beam Dec. 1986

142013/1/15 RIBF SEMINAR

Page 15: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Ring Cyclotron pamphlet 1986

152013/1/15 RIBF SEMINAR

Page 16: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Ring Cyclotron pamphlet 1990

GARIS/IGiSOL

RIPS

162013/1/15 RIBF SEMINAR

Page 17: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

172013/1/15 RIBF SEMINAR

Page 18: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Moved from RRC to RILAC facility

Layout of the RI Beam Factory (RIBF)

18

2000

2013/1/15 RIBF SEMINAR

Page 19: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

GARIS, GARIS-IICL

Superheavy Element Study at RIKEN RIBF

Experimental setups

Hot Lab.

192013/1/15 RIBF SEMINAR

Page 20: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

RILAC Facility 18GHz ECR Ion Source

RFQ-Linac

CSM   Acc. Tanks RILAC Acc. Tanks

GARIS

CSM Dec. Tank

202013/1/15 RIBF SEMINAR

Page 21: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 21

select the nuclei of ourinterest from the unwanted

then transport to thedetector chamber

Experimental setup

標的(金属薄膜)

incident ion beam(粒子の流れ)

イオン源

加速器

分離装置 (separator)

検出器 (detectors)

nucl. reaction

remove electrons from neutral atoms

accelerate ions using electric field information of energies or positionsof incoming ions and their decayparticles are transform to electric signal

18GHz ECR ion-source理研 original

RFQ-Linac

GARIS

Page 22: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

22

116115114

113112

111Ds

MtHs

BhSg

DbRfLrNoMd

EsCf

Fm

162

152

SFb+ or ECb-

170

176

Reactions studied at RIKEN-GARIS

277112 2 chains

271Ds 14 chains

272Rg 14 chains 278113

New !

208Pb(58Fe, n)265Hs208Pb(64Ni, n)271Ds209Bi(64Ni, n)272Rg208Pb(70Zn, n)277Cn209Bi(70Zn, n)278113207Pb(58Fe, n)264Hs206Pb(58Fe, n)263Hs208Pb(56Fe, n)263Hs208Pb(58Fe, 2n)264Hs248Cm(18O,5n)261Rf248Cm(22Ne,5n)265Sg248Cm(23Na,5n)266Bh

263, 264, 265Hs

261Rf

265Sg

2013/1/15 RIBF SEMINAR

Page 23: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

23

beamDifferential pumping section

D1Bending angle 45 degreePole gap 150 mmRadius of central ray 1200 mmMaximum field 1.54 TQ1, Q2Pole length 500 mmBore radius 150 mmMaximum field gradient 5.2 T/mD2Bending angle 10 degreePole gap 160 mmPole length 400 mmMaximum Field 1.04 T

Magnification X -0.76Y -1.99

Dispersion 0.97 cm/%Total length 5760 mmAcceptance ±68 mrad

f ±57 mradW 12.2 msr

Rotating Targetr 150 mmw 2000 rpm

RIKEN Gas-filled Recoil Separator GARIS

D1 Q1 Q2 D2

Standard method for heavy element physics: recoil separator + position sensitive FPD

2013/1/15 RIBF SEMINAR

Page 24: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

24

MCP1MCP2

SSD box

PSD

ions

Focal Plane Detectors

2013/1/15 RIBF SEMINAR

Page 25: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 25

Masses of Beams & TargetsAudi & Wapstra, Nucl. Phys A565, 1 (1993)

Masses of Compound NucleiMyers & Swiatecki, Nucl. Phys. A601, 141 (1996)

Calculated threshold of fission after 1n emission

5 10 15 20Ex of C.N. (MeV)

20

10

4

2

1

0.5

0.30.20.1

s (p

b)272Ds

273111

278112

279113

Page 26: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 26

Sn

(A – n) + n

A

B + T

B + T + EcmSn

saddle pointDeformation

Bf

Second chance fissionsreshold

saddle pointDeformation

Energy diagram of 1n emission

Ecm

Ex(

CN

)

Page 27: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Cold fusion:

208Pb 209Bi など魔法数をもつ安定な標的に相手方となるビームを照射する。クーロン障壁近傍の入射エネルギーでは複合核の励起エネルギーが15 ~ 20MeV 程度。複合核の脱励起の過程で 1 個ないし 2 個の中性子を出して超重元素である蒸発残留核を生じる。核分裂との競合回数が少ないのが利点であるが積 Z1 ・ Z2 が大きくいわゆる融合阻害の度合いが大きい。より中性子欠損の大きい核が合成されるため既知核へ連結することが多い。Hot fusion :アクチノイド標的に 48Ca を照射する。クーロン障壁近傍の入射エネルギーでは複合核の励起エネルギーが 35 ~ 45MeV 程度。 2 ないし 4 個の中性子を出して脱励起しする。cold fusion に比べて標的とビームの原子番号がより非対称であるため、積 Z1 ・ Z2 がcold fusion に比べ小さく、いわゆる融合阻害は無いと言われている。より中性子欠損が少ない核が合成され、 α 崩壊チェーンは中性子過剰な側に突っ込み既知核へ到達しない。

2013/1/15 RIBF SEMINAR 27

Page 28: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

RIBF SEMINAR

Cross-section systematics and extrapolation

300 fb 400 fb

23Na+248Cm => 266Bh+5n

Page 29: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 29

Page 30: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 30

Summary of 209Bi + 70Zn experiment

J. Phys. Soc. Jpn., Vol. 76 (2007) 045001J. Phys. Soc. Jpn., Vol. 73 (2004) 2593

period 2003/9/5 ~ 2012/8/18Beam Energy 5.03 AMeV

348 MeV at target half depth

Total Dose 1.35x1020

Target Thickness 1.3x1018 /cm2 (0.45 mg/cm2)e_GARIS 0.8s(3-events) 2.2x10-38 cm2

22 +20-13 fb

Irradiation time 13274 Hours (553 Days)Beam Intensity 2.8x1012 /s (0.47 p-mA)

J. Phys. Soc. Jpn., Vol. 81 (2012) 103201

Page 31: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

beamtime irradiation time

beam dose/sum

number of observed

eventsyear month/day [days] [×1019]2003 9/5 - 12/29 57.9 1.24/1.24 02004 7/8 - 8/2 21.9 0.51/1.75 12005 1/20 - 1/23 3.0 0.07/1.82 02005 3/20 - 4/22 27.1 0.71/2.53 12005 5/19 - 5/21 2.0 0.05/2.58 02005 8/7 - 8/25 16.1 0.45/3.03 02005 9/7 - 10/20 39.0 1.17/4.20 02005 11/25 - 12/15 19.5 0.63/4.83 02006 3/14 - 5/15 54.2 1.37/6.20 02008 1/9 - 3/31 70.9 2.28/8.48 02010 9/7 - 10/18 30.9 0.52/9.00 02011 1/22 - 5/22 89.8 2.01/11.01 02011 12/2 - 12/19 14.4 0.33/11.34 02012 1/15 - 2/9 25.0 0.56/11.90 02012 3/13 - 4/17 33.7 0.79/12.69 02012 6/12 - 7/2 15.7 0.25/12.94 02012 7/14 - 8/18 32.0 0.57/13.51 1Total 553 13.51 3

Table I. Summary of beamtime used.

2013/1/15 RIBF SEMINAR 31

Page 32: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 32

Page 33: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

2013/1/15 RIBF SEMINAR 33

278113

274111

270Mt

266Bh

CN11.68 MeV (PSD)344   μs30.49 mm

11.15 MeV6.149+5.003 (PSD+SSD)9.260 ms30.40 mm

10.03 MeV 1.136+8.894(PSD+SSD)7.163 ms29.79 mm

9.08 MeV (PSD)2.469 s30.91 mm

36.75 MeVTOF 44.61 ns30.33 mm

23-July-2004 18:55 (JST)

1st chain

262Db

204.05 MeV(PSD)40.9 s30.25 mm

278113

274111

270Mt

266Bh

CN11.52 MeV (PSD)4.93   ms30.16 mm

0.88+10.43=11.31 MeV(PSD+SSD)34.3 ms29.61 mm

2.32 MeV (escape)1.63 s29.45 mm

9.77 MeV (PSD)1.31 s29.65 mm

36.47 MeVTOF 45.69 ns30.08 mm

2-April-2005 2:18 (JST)

209Bi + 70Zn → 278113 + n

262Db

192.32 MeV(PSD)0.787 s30.47 mm

2nd chain

s.f.s.f.

s = 31 fb

Page 34: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

RIBF SEMINAR

266Bh267Bh262Db

200

150

100

50

250

E SF (D

augh

ter)

[MeV

]E

(Dau

ghte

r) [M

eV]

10

9

88 9 10

E (Mother) [MeV]

1-SF in (1-2-SF)2-SF in (1-2-SF)

J IH

G F E

2-3 in (1-2-3)1-2 in (1-2-3/SF)

1-3 in (1-2-3)1-2

1-SF

C A

B

D

a

b

262Db

258Lr

2013/1/15 34

Page 35: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

278113

274Rg

270Mt

266Bh

279113

262Db

267Bh 268Bh 269Bh 270Bh 271Bh

S.F.258Lr

one n evaporation

five n evaporation

decays observed in 278113 synthesis

decays observed in the present work 209Bi + 70Zn → 279113*

248Cm + 23Na → 271Bh*

2013/1/15 35RIBF SEMINAR

Page 36: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

362013/1/15 RIBF SEMINAR

Page 37: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

278113

274Rg

270Mt

266Bh

262Db

278113

274Rg

270Mt

266Bh

262Db

278113

274Rg

270Mt

266Bh

262Db

258Lr

254Md

1

2

3

4

S. F.

1

2

3

4

S. F.

1

2

3

4

5

6

Jul. 23, 2004Apr. 2, 2005

Aug. 12, 2012

11.68 ± 0.04 MeV0.344 ms

11.15 ± 0.07 MeV9.26 ms

10.03 ± 0.07 MeV7.16 ms

9.08 ± 0.04 MeV2.47 s

204 MeV40.9 s

11.52 ± 0.04 MeV4.93 ms

11.31 ± 0.07 MeV34.3 ms

2.32 MeV (escape)1.63 s

9.77 ± 0.04 MeV1.31 s

192MeV0.787 s

11.82 ± 0.06 MeV0.667 ms

10.65 ± 0.06 MeV9.97 ms

10.26 ± 0.07 MeV 444 ms

9.39 ± 0.06 MeV5.26 s

8.63 ± 0.06 MeV 126 s

8.66 ± 0.06 MeV3.78 s

2013/1/15 RIBF SEMINAR 37

Page 38: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

10 ms 1 ms 0.1 s 10 s 1000 s

278113 t = 2.0 ms

274Rg t = 18 ms

270Mt t = 0.69 s

266Bh t = 3.0 s

262Db t = 56 s

T_decay

previous

N=165

N=163

N=161

N=159

N=157

2013/1/15 RIBF SEMINAR 38

Page 39: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

10 ms 1 ms 0.1 s 10 s 1000 s

278113 t = 2.0 ms

274Rg t = 18 ms

270Mt t = 0.69 s

266Bh t = 3.0 s

262Db t = 56 s

T_decay

previous

N=165

N=163

N=161

N=159

N=157

present

2013/1/15 RIBF SEMINAR 39

Page 40: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

)exp(1)0()(tttNtn

)10lnexp(10 ut u

}]10ln)exp{(1[}]10ln)exp{(10ln)exp[()10)(ln0()(000

2 uuuuuuNduudn

崩壊時間の常用対数2013/1/15 RIBF SEMINAR 40

Page 41: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

254Fm(Z = 100):b = 99.94%, T1/2 = 3.240 ± 0.002 h6.898 ± 0.003 MeV (0.0066%),7.050 ± 0.002 MeV (0.82%),7.150 ± 0.002 MeV (14.2%),7.192 ± 0.002 MeV (84.9%).

254Md/ 254mMd(Z = 101):bEC = 100%/ 100%, T1/2 = 10 ± 3 / 28 ± 8 min

258Lr(Z = 103): b = 97.5%.T1/2 = 3.92+0.35

–0.42 s8.565 ± 0.025 MeV (20%), 8.595 ± 0.010 MeV (46%), 8.621 ± 0.010 MeV (25%),8.654 ± 0.010 MeV (9%)

262Db(Z = 105):b/bSF = 67%/33%.T1/2 = 34 ± 4 s8.450 ± 0.020 MeV (75%),8.530 ± 0.020 MeV (16%),8.670 ± 0.020 MeV (9%)

5

E = 8.63 ± 0.06 MeVt = 126 s (present)t = 56 +77 -21 s T1/2 = 39 +53 –14 s (three events)

6

E = 8.66 ± 0.06 MeVt = 3.78 s T1/2 = 2.6 +12 -1.1 s (one events)

no signal :E(X-ray of 254Fm)max = 142 keVEnergy threshold of PSD = 800 keV

7-1

E = 7.26 ± 0.07 MeVt = 3.96 h Pacc = 0.43

7-2

E = 7.18 ± 0.06 MeVt = 6.42 h Pacc = 0.70

250Cf (Z=98):b = 99.92%T1/2 = 13.08 y

2013/1/15 RIBF SEMINAR 41

Page 42: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

209Bi + 70Zn 278113 + n4: 266Bh (Z = 107)

1st E = 9.08 ± 0.04 MeV, t = 2.47 s2nd E = 9.77 ± 0.04 MeV, t = 1.31 s3rd E = 9.39 ± 0.06 MeV, t = 5.26 s

mean-life = 3.0 +4.2 -1.1 s T1/2 = 4.3 +6.1 -1.6 s

Cf:248Cm + 23Na 266Bh + 5n266Bh (Z = 107)

E = 9.05 - 9.23 MeV, t > s

2013/1/15 RIBF SEMINAR 42

Page 43: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

113

112 277Cn

111 272Rg

110 269Ds 270Ds 271Ds 273Ds

109 266Mt 268Mt

108 263Hs 265Hs 266Hs 267Hs 269Hs 270Hs 271Hs

107 261Bh 262Bh 264Bh 266Bh 267Bh

106 258Sg 259Sg 261Sg 263Sg

105 259Db 260Db

104 256Rf 260Rf 261Rf 262Rf

103 255Lr 257Lr 258Lr 259Lr 260Lr 261Lr 262Lr

102 256No 258No 260No 262No

101 253Md 254Md 259Md 260Md

100 252Fm 254Fm 255Fm 257Fm 258Fm 259Fm

99 251Es 253Es 256Es 257Es

98 250Cf 251Cf 252Cf 253Cf 254Cf 255Cf 256Cf

262Db

264Hs

265Sg 266Sg262Sg260Sg

263Db

263Rf

261Db257Db 258Db

257Rf 258Rf 259Rf

255Md 256Md 257Md 258Md

259No

256Fm253Fm

255No

256Lr

257No254No

252Es 255Es254ES

278113

274Rg

270Mt

266Bh

262Db

SF

278113

274Rg

270Mt

266Bh

262Db

258Lr

254Md

254Fm

250Cf

118

117 293117 294117

116

115 287115 288115 289115 290115

114

113 282113 283113 284113 285113 286113

278Rg 279Rg 280Rg 281Rg 282Rg

274Mt 275Mt 276Mt 278Mt

270Bh 271Bh 272Bh 274Bh

266Db 267Db 268Db 270Db

294118

290Lv 291Lv

286Fl 287Fl

282Cn

275Hs

267Rf

283Cn

279Ds

271Sg

1st event Jul. 23 20042nd event Apr. 2 20053rd event Aug. 12 2012

既知核種

FLNR/LLNR/GSI/LBNL

209Bi + 70Zn n

CN

2013/1/15 RIBF SEMINAR 43

Page 44: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

294118

290Lv 291Lv

286Fl 287Fl

282Cn 283Cn

275Hs

267Rf

271Sg

279Ds

113

112 277Cn

111 272Rg

110 269Ds 270Ds 271Ds 273Ds

109 266Mt 268Mt

108 263Hs 265Hs 266Hs 267Hs 269Hs 270Hs 271Hs

107 261Bh 262Bh 264Bh 266Bh 267Bh

106 258Sg 259Sg 261Sg 263Sg

105 259Db 260Db

104 256Rf 260Rf 261Rf 262Rf

103 255Lr 257Lr 258Lr 259Lr 260Lr 261Lr 262Lr

102 256No 258No 260No 262No

101 253Md 254Md 259Md 260Md

100 252Fm 254Fm 255Fm 257Fm 258Fm 259Fm

99 251Es 253Es 256Es 257Es

98 250Cf 251Cf 252Cf 253Cf 254Cf 255Cf 256Cf

262Db

264Hs

265Sg 266Sg262Sg260Sg

263Db

263Rf

261Db257Db 258Db

257Rf 258Rf 259Rf

255Md 256Md 257Md 258Md

259No

256Fm253Fm

255No

256Lr

257No254No

252Es 255Es254ES

278113

274Rg

270Mt

266Bh

262Db

278113

274Rg

270Mt

266Bh

262Db

258Lr

254Md

254Fm

250Cf

3rd event Aug. 12 2012

既知核種

118

117 293117 294117

116

115 287115 288115 289115 290115

114

113 282113 283113 284113 285113 286113

278Rg 279Rg 280Rg 281Rg 282Rg

274Mt 275Mt 276Mt 278Mt

270Bh 271Bh 272Bh 274Bh

266Db 267Db 268Db 270Db

FLNR/LLNR/GSI/LBNLActinide-based, 48Ca inducedHot fusion reactions

283113

279Rg

275Mt

271Bh

267Db

SF

287115

243Am + 48Ca 4n

284113

280Rg

276Mt

272Bh

268Db

SF

288115

243Am + 48Ca 3n

285113

281Rg

SF

289115

243Am + 48Ca 2n

282113

278Rg

274Mt

270Bh

266Db

SF

237Np + 48Ca 3n285113

281Rg

SF

289115

249Bk + 48Ca 4n

293117

286113

282Rg

278Mt

274Bh

270Db

SF

290115

294117

249Bk + 48Ca 3n

209Bi + 70Zn n

CN CN

CNCNCN

CNCN

2013/1/15 RIBF SEMINAR 44

Page 45: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

294118

290Lv 291Lv

286Fl 287Fl

282Cn

275Hs

267Rf

CN113

112 277Cn

111 272Rg

110 269Ds 270Ds 271Ds 273Ds

109 266Mt 268Mt

108 263Hs 265Hs 266Hs 267Hs 269Hs 270Hs 271Hs

107 261Bh 262Bh 264Bh 266Bh 267Bh

106 258Sg 259Sg 261Sg 263Sg

105 259Db 260Db

104 256Rf 260Rf 261Rf 262Rf

103 255Lr 257Lr 258Lr 259Lr 260Lr 261Lr 262Lr

102 256No 258No 260No 262No

101 253Md 254Md 259Md 260Md

100 252Fm 254Fm 255Fm 257Fm 258Fm 259Fm

99 251Es 253Es 256Es 257Es

98 250Cf 251Cf 252Cf 253Cf 254Cf 255Cf 256Cf

262Db

264Hs

265Sg 266Sg262Sg260Sg

263Db

263Rf

261Db257Db 258Db

257Rf 258Rf 259Rf

255Md 256Md 257Md 258Md

259No

256Fm253Fm

255No

256Lr

257No254No

252Es 255Es254ES

278113

274Rg

270Mt

266Bh

262Db

278113

274Rg

270Mt

266Bh

262Db

258Lr

254Md

254Fm

250Cf

3rd event Aug. 12 2012

既知核種

118

117 293117 294117

116

115 287115 288115 289115 290115

114

113 282113 283113 284113 285113 286113

283Cn

278Rg 279Rg 280Rg 281Rg 282Rg

274Mt 275Mt 276Mt 278Mt

270Bh 271Bh 272Bh 274Bh

266Db 267Db 268Db 270Db

FLNR/LLNR/GSI/LBNLActinide-based, 48Ca inducedHot fusion reactions

249Bk + 48Ca 4n

243Am + 48Ca 2n

209Bi + 70Zn n

285113

281Rg

SF

289115

285113

281Rg

SF

289115

293117

CN

CN

279Ds

271Sg

2013/1/15 RIBF SEMINAR 45

Page 46: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

46

1.E-01

1.E+00

1.E+01

1.E+02

1.E+03

156 158 160 162 164 166

112113113-2Hi

ndra

nce

Fact

or (T

exp/

T calc)

dcZQbaZTcalc 10log

Systematics by Viola & Seaborg

a=1.81040, b=-21.7199, c=-0.26488, d=-28.1319by Smolanczuk, Phys. Rev. C56(1997)812

112DsHs

SgRf

113

RgMtBh

neutron number

1661641621601580.1

156

1

10

100

1000

2013/1/15 RIBF SEMINAR

Page 47: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

Program of SHE search and spectroscopy209Bi(70Zn, n)278113 experiment completed on Oct. 1, 2012.Study 208Pb(76Ge, n)283114(Fl) reaction (under discussion).Start 248Cm(54Cr, 3n)299120 experiment.Systematic study of 50Ti induced hot-fusion reactions 248Cm(48Ca, 3n)293Lv244Pu(50Ti, 3n)291Lv248Cm(50Ti, 3n)295118

New isotope search of the heaviest nuclei and detailed spectroscopy with cold and hot fusion reactions.

Mass measurement of the heaviest nuclei with m-TOF system coupled to GARIS (Wada-san’s group)

Study of heavy ion transfer reaction with GARIS for the study of neutron rich nuclei around N=126 region.

Try to measure X-ray from evaporation residues (in collaboration with W. Henning).

Developing FPD detector system for --e coincidence experiment

472013/1/15 RIBF SEMINAR

Page 48: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

48

RIKEN Nishina CenterH. Haba, H. Hasebe, D. Kaji, K. Katori, Y. Kudou,

T. Ohnishi, K. Ozeki, K. Morimoto, A. Yoneda, A. Yoshida,

Tokyo University of ScienceT. Sumita, K. Tanaka, J. Chiba

Saitama University

T. Akiyama, R. Sakai, S. Yamaki, T. Yamaguchi

Tohoku UniversityT. Suda, H. Kikunaga, T. Shinozuka

JAEA

H. Koura, S. Mitsuoka, K. Ooe, N. Sato, A. Toyoshima, K. Tsukada, Y. Wakabayashi

Niigata University

S. Goto, M. Murakami, M. Murayama, Y. Kanaya, H. Kudo,

YITP Kyoto University

T. Ichikawa,

University of TsukubaA. Ozawa, K. Sueki

Yamagata University

Y. Fujimori, K. Mayama, T. Mashiko ,S. Namai, M. Takeyama, F. Tokanai,

Center for Nuclear Science, University of Tokyo

E. Ideguchi

Osaka UniversityY. Kasamatsu, Y. Kitamoto, Y. Komori, T. Kuribayashi,

K. Matsuo, D. Saika, A. Shinohara, T. Takabe, Y. Tashiro, T. Yoshimura

Kanazawa University

T. Nanri, D. Suzuki, I. Yamazaki, A. Yokoyama

Collaborators (2006 - )

2013/1/15 RIBF SEMINAR

Page 49: New Result in Production and Decay of an Isotope,  278 113, of the 113 th  Element  Kosuke Morita

49

Thank you very much for your kind attention!

2013/1/15 RIBF SEMINAR