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Tatsushi Shima Research Center for Nuclear Physics, Osaka University 日本物理学会/山形大学/2008920超新星爆発に関与する光核反応の実験的研究 超新星爆発に関与する光核反応の実験的研究 Experimental Study of Photonuclear Reactions Experimental Study of Photonuclear Reactions Relevant to Supernova Explosions Relevant to Supernova Explosions Photonuclear reactions related to SNe Laser Compton-scattered γ-ray source Recent experiment; ex. 4 He Summary & Outlook

Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

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Page 1: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Tatsushi ShimaResearch Center for Nuclear Physics, Osaka University

日本物理学会/山形大学/2008年9月20日

超新星爆発に関与する光核反応の実験的研究超新星爆発に関与する光核反応の実験的研究

Experimental Study of Photonuclear ReactionsExperimental Study of Photonuclear ReactionsRelevant to Supernova ExplosionsRelevant to Supernova Explosions

Photonuclear reactions related to SNeLaser Compton-scattered γ-ray sourceRecent experiment; ex. 4HeSummary & Outlook

Page 2: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

He-burning ; 12C(α,γ)16O ⇔ 16O(γ,α)12C (detailed balance)

Photodisintegration of iron core ;

(γ,α), 4He(γ,p)3H(γ,n)2H(γ,n)1H, 4He(γ,n)3He(γ,p)2H(γ,n)1H

r-, p-, γ-processes ; (p,γ), (n,γ), (γ,n), (γ,p), (γ,α)

ν-process ; (ν,ν’x) (neutral current) ⇔ (γ,x)

--- nuclear responses to dipole excitation by τ3, σ·τ3

Photonuclear Reactions Related to Photonuclear Reactions Related to Supernova ExplosionsSupernova Explosions

Page 3: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Photonuclear reactionsPhotonuclear reactionsas a tool for nuclear astrophysicsas a tool for nuclear astrophysics

EM interaction; well-know !

Sensitivity to multi-body channels; X+Y+Z+…→A+γ ⇔ A+γ → X+Y+Z+…ex. 2α+n → 9Be, 3α → 12C

Enhancement of cross sections by phase space factor

Analogy between γ-A and ν-A interactions

Page 4: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

LowLow--energy energy γγ--ray sources ray sources Discrete γ-rays from radioisotopes

Bremsstrahlung (continuous energy) / tagged photons

e+e- pair annihilation in flight ; monoenergy γ + brems.

Laser Compton Scattered γ (LCS-γ)Synchrotron photons from super-conducting wiggler

--- quasi-Planck spectrum (Utsunomiya, Nucl. Phys. A777)

Coulomb Dissociation (CD) ; virtual photons, application to RI7Be(p,γ)8B, 14C(n,γ)15C, … RIKEN, GSI

(p,p’) ; probe for M1 excitation RCNP

Page 5: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Laser Compton backscatteringLaser Compton backscattering

Relativistic electron (Ee)

Laser light (λL)

γ (Eγ)

222

2

, 1

4cm

EhcEe

e

L

=+

⋅= γθγ

γλγ

ex. λL=1.064μm, Ee=974MeV⇒ Eγ = 17MeV

E γ [M

eV]

θ [mrad]

Ee=0.974GeV, λL=1064nm

0 0.5 1 1.5 2

5

10

15

20

Page 6: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Energy distributionsEnergy distributions

Bremsstrahlung,e+e- annihilation in flight

Laser Compton-Scattered γ(PH spectra of GSO scintillator)

Pulse Height [MeV]

Cou

nt [

arb.

uni

t] λ laser =1064nm, Ee = 0.976GeV, Ie =83mA

Plaser=3.53WPlaser=0W

0 5 10 15 20

100

200

No BG !!BG from low-energy component of brems.

Page 7: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Energy distributionEnergy distribution

NaI(Tl): 6”φ×5”Collimator: φ3mm

FWHM 8.7%

DataFitEγ

Eγ(max) = 34MeV

Eγ [MeV]

Cou

nt

0 8 16 24 32 40

40

80

120

Page 8: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Advantages of LCSAdvantages of LCS--γγ

Quasi-monochromatic; ΔE/E < ~10%, little BG

Well-collimated; Δθ < 0.1 mrad

Highly polarized; linear or circular, P ~ 100%

Continuous or pulsed; Δt < 10ns

Page 9: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

LCS LCS γγ--ray facilities in the worldray facilities in the world

Year Facility Ee

[GeV]Laser Eγ

[MeV]Φγ

[/sec/MeV]1964 Lebedev 0.6 ruby ~10 ~ 106

1965 Harvard / CEA 6 ruby ~1000 5×104

1978 Frascati / LADON 1.5 Ar+ 5 - 80 ~ 105

1985 ETL(AIST) / TERAS 0.2-0.8 Nd-YAG 2 - 40 103 ~105

1990 BNL / LEGS 2.8 Nd-YAG 150 - 470 104 ~ 105

1996 Grenoble / GrAAL 6 Ar+ 1500 ~ 4×103

1999 SPring-8 / LEPS 8 Ar+ 1500 - 3500 ~104

1999 TUNL(Duke) / HIγS 0.2-1.2 FEL 2 - 70 ~ 107

2004 LASTI(U. Hyogo) / NewSUBARU

1 - 1.5 Nd-YVO4 16 - 40 104 ~ 105

Page 10: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Injection BTS

RF cavity

Septum

Kicker

QF

QD

QFElectron storage ring, “TERAS”:300 – 800 MeV, 300 mA

0 1 m 2 m

laser

light

LCS be

am

1 ~ 40

MeV

LCS-3

e-

AIST/LCS AIST/LCS γγ--sourcesource産総研(つくば)

Page 11: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Duke/Duke/HIgSHIgS ((High Intensity High Intensity γγ--ray Sourceray Source))

Intra-cavity Compton Backscattering of FEL photons by electrons circulating in the 1.2GeV Duke Storage Ring

Eγ = 2~70 MeV, ΔEγ/Eγ ~ 1%, Φγ ~ 107 /MeV/s (→ 109 )

Time interval of γ-ray pulses ; 170ns

Page 12: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

NewSUBARUNewSUBARU Lab. of Adv. Sci. and Tech. for Industry, University of Hyogo, Japan

Page 13: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

SubaruSubaru is an old Japanese meaning “get together”, and also the Japanese name of the Pleiades Star Cluster.

Subaru NewSUBARU SUBARU

Type Telescope SR facility AutomakerLocation Mauna Kea, Hawaii Hyogo, Japan Gunma, Japan

Feature8.2m single mirror with adaptive optics

Race-track shape isochronous ring

Boxer engine + symmetrical AWD

Memorial First light 1999 First beam 1998 WRC first win 1993

Page 14: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

NewSUBARU/LCSNewSUBARU/LCS--γγ sourcesource

Linac

e-

1.0GeV

K. Aoki, S. Miyamoto, et al. NIM A516 (2004) 228-236

Eγ =16 - 40 MeV, Φγ =104~5 photons/MeV/s, ΔEγ/Eγ =3~10%

“Top-up” mode⇓

stable Eγ , Φγ

Page 15: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Merits of Merits of NewSUBARUNewSUBARU LCS LCS γγ--sourcesource

Conventional lasers (Nd:YVO4, CO2, etc.) are used.

→ Various kinds of lasers can be employed.

Flexibility in energy range, pulse structure,

polarization, etc.

Laser and electron beam collide in a straight section.

→ Little background from bremsstrahlung

Top-up (top-loaded) operation is available.

→ High flux and excellent stability

Page 16: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

44He(He(γγ,X) ,X) ⇔⇔ 44He(He(νν,,νν’’))

Neutrino-heating effect needs CS with 10% accuracy

R-process in neutrino-driven wind

without 4He(ν,ν’) with 4He(ν,ν’)

Meyer, ApJ449 (1995) L55

Page 17: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

4He(ν,ν’p)3H(α,γ)7Li(α,γ)11B4He(ν,ν’n)3He(α,γ)7Be(e-,νe)7Li

77Li, Li, 1111B production by B production by νν--spallationsspallationsWoosley et al., Woosley & Weaver, Rauscher et al., Yoshida et al.

Yoshida, Kajino et al., PRL96, 091101 (2006)

Page 18: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Neutrino neutral reaction rate on Neutrino neutral reaction rate on 44HeHe

Tν [MeV]

<σ>

[10-4

2 cm

2 ]

Woosley, Haxton 1990 (shell model)Gazit, Barnea 2004 (Lorentz Int.)

4 6 8 10 120

0.5

1

1.5

2

Page 19: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

ShellShell--model calculationmodel calculationT. Suzuki et al., PR C74 034307 (2006)

Page 20: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

4He(γ,p)3H

0

1

2

4He(γ,n)3He

Cro

ss S

ectio

n [m

b]

Eγ [MeV]20 30 40 500

1

2

Photodisintegration of 4He have been studied by means ofmonochromatic γ, bremsstrahlung, radiative capture...

Page 21: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Experiment at Experiment at NewSUBARUNewSUBARU LCSLCS--γγ facilityfacility

Eγ = 16 ~ 40MeV, Φγ =2~4×104 /sec, FWHM~9%, P~100%

Page 22: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Time Projection ChamberTime Projection Chamber

Target gas : He + CD4

--- active target

· Ω ~ 4π , ε > 98% ; high efficiency · track shape, dE/dx ⇒ event ID, dσ/dΩ, asymmetry

T. Kii, T. Shima, T. Baba, Y. Nagai, NIM A552 (2005) 329

Page 23: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Event IdentificationEvent Identification

4He(γ,p)3H

4He(γ,n)3He

4He photodisintegrationsx

[mm

]

z [mm]

γ-beam

p

3H0 50 100 150 200 250-30

0

30

x [m

m]

z [mm]

γ-beam

3He

0 50 100 150 200 250-30

0

30

Page 24: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

12C photodisintegrations

12C(γ,p)11B

12C(γ,n)11C

x [m

m]

z [mm]

γ-beam 11B

p

0 50 100 150 200 250-30

0

30

x [m

m]

z [mm]

γ-beam

11C

0 50 100 150 200 250-30

0

30

Page 25: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Three-body decays

4He(γ,pn)2H

12C(γ,2α)4He

x [m

m]

z [mm]

γ-beam

d

p0 50 100 150 200 250-30

0

30

x [m

m]

z [mm]

γ-beam

α α

α

0 50 100 150 200 250-30

0

30

Page 26: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Backgroundsx

[mm

]

z [mm]0 50 100 150 200 250-30

0

30

x [m

m]

z [mm]0 50 100 150 200 250-30

0

30

α from natural RI

Photoelectrons

Page 27: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

D(γ,p)n

x [m

m]

z [mm]

γ-beam p0 50 100 150 200 250-30

0

30

Page 28: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

44He(He(γγ,p),p)33H H (preliminary)(preliminary)

●○ RCNP-AIST (PRC72, 044004) ; λ=351nm (3rd), Ee=0.8GeV●○ RCNP-AIST (PRC72, 044004) ; λ=351nm (3rd), Ee=0.8GeV● RCNP-NewSUBARU; λ=532nm (2nd), Ee=0.97GeV● RCNP-NewSUBARU; λ=1064nm (fund.), Ee≤1.46GeV

●○ RCNP-AIST (PRC72, 044004) ; λ=351nm (3rd), Ee=0.8GeV● RCNP-NewSUBARU; λ=532nm (2nd), Ee=0.97GeV● RCNP-NewSUBARU; λ=1064nm (fund.), Ee≤1.46GeV○ RCNP-NewSUBARU; λ=532nm (2nd), Ee=1.06GeV

Eγ [MeV]

Cro

ss S

ectio

n [m

b]

20 25 30 35 40 45 500

1

2

Eγ [MeV]

Cro

ss S

ectio

n [m

b]

20 25 30 35 40 45 500

1

2

Eγ [MeV]

Cro

ss S

ectio

n [m

b]

20 25 30 35 40 45 500

1

2

Page 29: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

44He(He(γγ,n),n)33He He (preliminary)(preliminary)

Eγ [MeV]

Cro

ss S

ectio

n [m

b]

20 25 30 35 40 45 500

1

2

●○ RCNP-AIST (PRC72, 044004) ; λ=351nm (3rd), Ee=0.8GeV● RCNP-NewSUBARU; λ=532nm (2nd), Ee=0.97MeV● RCNP-NewSUBARU; λ=1064nm (fund.), Ee≤1.46GeV○ RCNP-NewSUBARU; λ=532nm (2nd), Ee=1.06GeV

● Lund 2005-2007 (PRC75, 014007) ; tagged photons

Page 30: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

44He(He(γγ,pn)d ,pn)d (preliminary)(preliminary)

Eγ [MeV]

Cro

ss S

ectio

n [m

b]

Gorbunov1958Arkatov1969Balestra1979RCNP-AISTRCNP-NewSUBARU (1)RCNP-NewSUBARU (2)RCNP-NewSUBARU (3)

Threshold26.07MeV

28 32 36 400

0.1

0.2

0.3

0.4

Page 31: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Eγ [MeV]

Cro

ss S

ectio

n [m

b]Skopik 74Bernabei 86Leleux 79,85Michel 89RCNP-AISTRCNP-NewSUBARU (1)RCNP-NewSUBARU (2)RCNP-NewSUBARU (3)

ENDF/B-VIIPartovi 1964

10 15 20 25 30 35 400

0.4

0.8

1.2

D(D(γγ,n)p,n)p

Page 32: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

SummarySummaryLaser Compton Scattered γ, combined with new detector

techniques, provides a useful tool for high-precision studies of nuclear reactions induced by photons and also neutrinos.

Complementary to radiative capture, CD, (p,p’), ...

The LCS γ-source at NewSUBARU is now in operation, and several works for nuclear astrophysics have been performed

successfully.

4He: excitation functions are measured up to 37MeV. Small cross sections below 30MeV were confirmed.

GDR peak was found to locate at ~32.5MeV. → → → p-n, 1p1h, 3NF

Other light nuclei and heavier p-nuclei are planned to be studied.

Page 33: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

OutlookOutlook(γ,n) cross sections of long-lived radioactive nuclide ;

Φγ =104 /s ⇒ 106 /s ; target: 1g ⇒ 10mg

(γ,p), (γ,a) cross sections of p-nuclei ;

for noble gases --- TPC

for others --- activation method

Reference data for indirect methods ; CD, (p,p’), ...

Technical hint for experiment with other neutral beams ; n, ν

Page 34: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Present; Nd:YVO4 laser (1.06μm), 1W ⇒ Eγ =16.5MeV, Φγ ~ 3×104 photons/s

Plan; Tm-doped fiber laser (2.05μm), 100W⇒ Eγ =8.5MeV, Φγ > 106 photons/s

Page 35: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Neutron detector for (Neutron detector for (γγ,n,n) (Konan Univ.)) (Konan Univ.)

4π long counters

Beam dump (NaI(Tl) detector)

Page 36: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Utsunomiya et al., PRC74 025806 (2006)

Page 37: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

Radioactivity < 1MBq, 100μmol T1/2 > ~10000yr

β±-γ, T1/2>104y (15 nuclides) ; 10Be, 26Al, 36Cl, 40K, 59Ni, 79Se, 93Zr, 92Nb, 98,99Tc, 107Pd, 135Cs, 138La, 186Re, 208Bi

EC, no γ, T1/2>100d (12 nuclides) ;41Ca, 49V, 53Mn, 55Fe, 93Mo, 97Tc, 109Cd, 137La, 179Ta, 178W, 193Pt, 205Pb

α-γ, T1/2>104y (16 nuclides) ;210Bi, 230,232Th, 231Pa, 233-236,238U, 236,237Np, 239,242,244Pu, 247,248Cm

α, no γ, T1/2>100d (4 nuclides) ; 146Sm, 148,150Gd, 154Dy

Page 38: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

OutlookOutlook(γ,n) cross sections of long-lived radioactive nuclide ;

Φγ =104 /s ⇒ 106 /s ; target: 1g ⇒ 10mg

(γ,p), (γ,a) cross sections of p-nuclei ;

for noble gases --- TPC

for others --- activation method

Reference data for indirect methods ; CD, (p,p’), ...

Technical hint for experiment with other neutral beams ; n, ν

Page 39: Experimental Study of Photonuclear Reactions Relevant to ...shima/Ukakuren/ws/JPS2008a/Shima.pdfnuclear reactions induced by photons and also neutrinos. Complementary to radiative

CollaboratorsCollaboratorsH. Utsunomiya, H. Akimune

Department of Physics, Konan University

T. Mochizuki, S. Miyamoto, K. HorikawaLaboratory for Advanced Science and Technology for Industry, University of Hyogo

T. Hayakawa, T. ShizumaKansai Photon Science Institute, Japan Atomic Energy Agency

M. FujiwaraResearch Center for Nuclear Physics, Osaka University

Y. NagaiNuclear Science and Engineering Directorate, Japan Atomic Energy Agency